Airborne Laser Infrared Absorption Spectrometer (ALIAS-II)


 

Instrument:Airborne Laser Infrared Absorption Spectrometer (ALIAS-II)
Principal Investigator:Christopher R. Webster
Co-Investigator:David C. Scott and Robert L. Herman
Organization:National Aeronautics and Space Administration
Jet Propulsion Laboratory
4800 Oak Grove Drive
Pasadena, CA 91109-8099

Plot of Amplitude vs wave number image of the ALIAS II instrument

Measurement Description: The Airborne Laser Infrared Absorption Spectrometer (ALIAS-II) is a very high resolution scanning tunable diode laser spectrometer which makes direct, simultaneous measurements of selectable combinations of HCl, NO2, CO, CO2, CH4, and N2O at sub-part-per-billion levels over a 3-30 second integration time. The measurement technique is based upon using tunable lead-salt and/or quantum cascade lasers operating from 3.4 to 8 microns wavelength scanning over absorption lines at 10 Hz recording second harmonic spectra. The instrument features an open-cradle multipass Herriott absorption cell with 15.24-cm diameter spherical zerodur mirrors coated with gold on chrome. The separation between the mirrors is adjustable allowing for a relatively small cell (0.75-m to 1.5-m) to contain an optical path length up to 120-m, depending on the spacing of the mirrors. Lasers and detectors are contained in a lightweight aluminum liquid nitrogen Dewar which can achieve a 28-hour hold time with only a 2 liter charge of liquid nitrogen. The instrument features custom laser current drives, signal chains, InSb detectors and preamps, 16-bit signal averager, analog signal conditioner, and digital I/O which are controlled by an onboard Pentium processor. Data is written to a ruggedized 2-Gb hard disk every 30 seconds and simultaneously transmitted via telemetry to ground station computers which provide backup storage of the data. The instrument weighs 36 kg. and requires <56 watts for operation. Additional power up to 250 watts is available for structural heaters and current draw varies with atmospheric conditions. For launch on the Jet Propulsion Laboratorys Observations from the Middle Stratosphere gondola the optical assembly is deployed outside the gondola to sample free stream air and the electronics remain inside the gondola. Before the flight is terminated the optical assembly is retracted and stowed to withstand up to 10-Gs. ALIAS-II has flown successfully on seven missions out of Ft. Sumner, New Mexico, Fairbanks, Alaska, and Juazeiro do Norte, Brazil.

Accuracy:Typically 2-10%, depending upon calibration gases and IR spectral parameters.
Precision:Typically 2-10%, depending upon SNR for observed atmospheric concentration.
Detection Limits:HCl and NO2 (0.03 ppbv): N2O, CH4, and CO (0.1ppbv).
Response Time:3-30 seconds depending upon SNR for observed atmospheric concentration.

 

References:

Herman, R. L., D. C. Scott, C. R. Webster, R. D. May, E. J. Moyer, R. J. Salawitch, Y. L. Yung, G. C. Toon, B. Sen, J. J. Margitan, K. H. Rosenlof, H. A. Michelsen, and J. W. Elkins, Tropical entrainment timescales inferred from stratospheric N2O and CH4 observations, Geophys. Res. Lett., 25, 2781-2784, 1998.
Scott, D. C., R. L. Herman, C. R. Webster, R. D. May, G. J. Flesch, and E. J. Moyer, Airborne Laser Infrared Absorption Spectrometer (ALIAS-II) for in situ atmospheric measurements of N2O, CH4, CO, HCl, and NO2 from balloon or remotely piloted aircraft platforms, Appl. Optics, 38, 4609-4622, 1999.